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Effects of molecular conformation on buried interface passivation and efficient perovskite solar cell realization employing fluorine substituted benzoic acid 认领 引用
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作者 Boyan Li Rongbo Wang +8 位作者 Ya Wang Wentao Wu Weitao Yan Handong Zhang Xingyuan Zhong Juntao Zhao Liyi Yao Wei-Hua Wang Yi Ding 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2026年第1期826-831,I0018,共6页
Benzoic acid containing fluorine atom at ortho-,meta-,and para-position are employed as self-assembled monolayers to modify the buried interface in perovskite solar cells(PSCs).It is demonstrated that the position of ... Benzoic acid containing fluorine atom at ortho-,meta-,and para-position are employed as self-assembled monolayers to modify the buried interface in perovskite solar cells(PSCs).It is demonstrated that the position of fluorine atom influences the passivation effect and para-fluorinated one provided the most substantial performance enhancement mainly originating from ameliorated contact and energy band alignment between NiOx and perovskite,improved perovskite quality and defect healing.Resultantly,PSC with a power conversion efficiency of 24%can be achieved.Meanwhile,which can maintain 96.8%of the initial PCE after a 1000 h storage,presenting enhanced durability.This work highlights the critical role of molecular functionality and conformation in the buried interface modification of PSCs,providing valuable insights for future developments. 展开更多
关键词 Perovskite solar cells F atom substituted benzoic acids Buried interface modification
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