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Reactive nano-essential oils for sustained release of essential oils and application to wallpaper 认领 引用 被引量：4
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作者 Qiulian Hao Huan Peng +9 位作者 Ruichen Zhao Jianze Wang Zhiguo Lu Jingwen Wang Jie Shen Yunwei Niu Zuobing Xiao Guiying Liu Jifu Hao Xin Zhang 《Chinese Chemical Letters》 SCIE CAS CSCD 2022年第1期320-323,共4页
Essential oils are a volatile and aromatic substance with a variety of active biological activities.However,the excessive volatility and inconvenience of the use of essential oils limit their applications.In this stud... Essential oils are a volatile and aromatic substance with a variety of active biological activities.However,the excessive volatility and inconvenience of the use of essential oils limit their applications.In this study,we developed a reactive mesoporous silica nanoparticle(rMSNs)based on cyanuric chloride modification for essential oil encapsulation and commodity adhesion.The large pore volume and specific surface area of rMSNs facilitate the nanoparticles adhering to a large amount of essential oil and achieve the sustained release of essential oil,thus prolonging the fragrance retention time of essential oils.The reactive nanoessential oils can form covalent bonds with the wallpaper,thereby remarkably improving the adhesion of the reactive nano-essential oils on the wallpaper and preventing the reactive nano-essential oil from deadhering from the wallpaper.The active nano essential oil simultaneously overcomes the intense volatility of the essential oil and inconvenience in use,has a simple preparation process and low cost,and has great application potential. 展开更多
关键词 Reactive nano-essential oils Reactive mesoporous silica nanoparticles Slow-release of essential oils Application to wallpaper Covalent bonds
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Preparation of mesoporous silica nanoparticle with tunable pore diameters for encapsulating and slowly releasing eugenol 认领 引用 被引量：4
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作者 Tianlu Zhang Zhiguo Lu +8 位作者 Jianze Wang Jie Shen Qiulian Hao Yan Li Jun Yang Yunwei Niu Zuobing Xiao Lei Chen Xin Zhang 《Chinese Chemical Letters》 SCIE CAS CSCD 2021年第5期1755-1758,共4页
Fragrances are frequently added to a variety of products,including food,cosmetics and health products.However,the high volatility and instability of essence limit its application in some fields.In this study,mesoporou... Fragrances are frequently added to a variety of products,including food,cosmetics and health products.However,the high volatility and instability of essence limit its application in some fields.In this study,mesoporous silica nanoparticles(MSNs) were prepared to encapsulate eugenol,which could reduce the volatilization of the fragrance molecules.A facile approach was presented to synthesize MSNs with three different pore diameters for encapsulating eugenol.In addition,the properties of MSNs including mean particle size,morphology,encapsulating efficiency and release tendency were charac terized.Results showed that the larger the pore diameters of MSNs,the more aromatic molecules were adsorbed.Furthermore,the release mechanism was described as the smaller the pore diameters of MSNs,the slower the release of eugenol. 展开更多
关键词 Eugenol Mesoporous silica nanoparticles Nano-fragrance Slow release of fragrance
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Zwitterionic comb-like lipid polymers encapsulating linalool for increasing the fragrance retention time 认领 引用 被引量：2
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作者 Tianlu Zhang Zhiguo Lu +5 位作者 Xiangyu Wang Jie Shen Jianze Wang Yunwei Niu Zuobing Xiao Xin Zhang 《Chinese Chemical Letters》 SCIE CAS CSCD 2021年第1期573-576,共4页
Fragrances are widely used in cosmetics,apparel and detergents.However,the rapid evaporation of the aro ma shortens the useful life of the aromatic product.Therefore,improving the fragrance retention time of aromatic ... Fragrances are widely used in cosmetics,apparel and detergents.However,the rapid evaporation of the aro ma shortens the useful life of the aromatic product.Therefore,improving the fragrance retention time of aromatic products and prolonging the service life of aromatic products are the key scientific problems that need to be solved in current aromatic products.In this study,zwitterionic comb-like lipid polymers were synthesized to encapsulate the fragrance molecule linalool.The results showed that the zwitterionic comb lipid molecules were capable of encapsulating more linalool than linear lipid molecules.At the same time,the zwitterionic comb-like lipid molecules also limited the slow release rate of the aroma,thereby increasing the fragrance retention time of the nano-fragrance. 展开更多
关键词 Linalool Zwitterionic comb-like lipid polymers Nano-fragrance Fragrance retention time Slow release
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Mesoporous silica nanospheres with the ability of photo-driven releasing sandela 803 for the application to wallpaper 认领 引用 被引量：1
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作者 Weihong Ji Tianlu Zhang +5 位作者 Zhiguo Lu Jie Shen Jing Hu Yunwei Niu Zuobing Xiao Xin Zhang 《Chinese Chemical Letters》 SCIE CAS CSCD 2019年第3期747-749,共3页
Fragrances are widely used in our daily life and have made great contributions to creating a clean and fresh healthy air environment. However, the rapid volatilization severely influences their storage,application and... Fragrances are widely used in our daily life and have made great contributions to creating a clean and fresh healthy air environment. However, the rapid volatilization severely influences their storage,application and quality. Therefore, it is necessary and urgent to develop approaches to controllably release the odorants as demanded. In this study, photo-driven mesoporous silica nanospheres loaded with sandela 803 was designed, prepared and named as S803@MS-S. S803@MS-S possessed ordered mesoporous, large specific surface area and pore volume. After adsorption of sandela 803, the S803@MSS was added into wallpaper to prepare fragrant wallpaper S803@MS-S-W. And this wallpaper exhibited excellent sustained and controlled release performances stimulated by light. 展开更多
关键词 Mesoporous silica nanospheres Sandela 803 Photo-driven release Wallpaper Azobenzene derivatives
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Cationic and temperature-sensitive liposomes loaded with eugenol for the application to silk 认领 引用
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作者 Zhiguo Lu Xiangyu Wang +9 位作者 Tianlu Zhang Luyao Zhang Jun Yang Yan Li Jie Shen Jianze Wang Yunwei Niu Zuobing Xiao Guiying Liu Xin Zhang 《Chinese Chemical Letters》 SCIE CAS CSCD 2020年第12期3139-3142,共4页
Silk has been widely used in the clothing industry due to their soft and smooth features,good biocompatibility,good heat dissipation,warmth and ultraviolet resistance.The application of fragrance to silk can significa... Silk has been widely used in the clothing industry due to their soft and smooth features,good biocompatibility,good heat dissipation,warmth and ultraviolet resistance.The application of fragrance to silk can significantly improve the performance of silk.However,there are two key scientific problems that need to be solved:slowing down the release rate of fragrances and increasing the scent lasting time of silk.In this study,cationic and temperature-sensitive liposomes were designed and prepared to encapsulate eugenol.These fragrance-loaded liposomes significantly slowed down the release rate of the fragrance and controlled the release rate of the fragrance in a thermo-sensitive manner.The liposomes adhered to the silk through electrostatic adsorption interaction.The positive charge on the fragranceloaded liposomes neutralized much negative charge on silk and thereby increasing the adhesion efficiency. 展开更多
关键词 Eugenol Silk Cationic and temperature-sensitive liposomes Slow release of fragrance Controlled release of fragrance
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Preparation of hollow mesoporous silica nanorods for encapsulating and slowly releasing eugenol 认领 引用
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作者 Tianlu Zhang Zhiguo Lu +8 位作者 Luyao Zhang Yan Li Jun Yang Jie Shen Jianze Wang Yunwei Niu Zuobing Xiao Lei Chen Xin Zhang 《Chinese Chemical Letters》 SCIE CAS CSCD 2020年第12期3135-3138,共4页
Fragrances are widely used in many aspects of our lives.They cannot only make people happy,but also treat many diseases.However,excessively fast evaporation rate is one of the main obstacles to the use of spices.In th... Fragrances are widely used in many aspects of our lives.They cannot only make people happy,but also treat many diseases.However,excessively fast evaporation rate is one of the main obstacles to the use of spices.In this study,mesoporous silica nanorods(MSNRs)and hollow mesoporous silica nanorods(HMSNRs)were prepared to encapsulate eugenol.These two nano-fragrances were named eugenol@MSNRs and eugenol@HMSNRs,respectively.The morphologies,size,interior structures and pore performances of MSNRs and HMSNRs.Besides,the performances of encapsulation and fragrance release of eugenol@MSNRs and eugenol@HMSNRs were compared and analyzed.The results showed that eugenol@HMSNRs encapsulated more fragrance and were faster to encapsulate compared with eugenol@MSNRs.Both the release rates of eugenol from eugenol@MSNRs and eugenol@HMSNRs were slow.But the eugenol was released from eugenol@MSNRs more slowly. 展开更多
关键词 Eugenol Hollow mesoporous silica nanorods Mesoporous silica nanorods Nano-fragrance Slow release of fragrance
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Biodegradable Materials as Nanocarriers for Drugs and Nutrients 认领 引用
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作者 Xingran Kou Qixuan Zhao +3 位作者 Wenwen Xu Zuobing Xiao Yunwei Niu Kai Wang 《Journal of Renewable Materials》 SCIE EI CAS 2021年第7期1189-1211,共23页
Several important drugs and nutritional supplements are limited by their lack of bioavailability.Nanomaterials display unique beneficial properties that might help improve the bioavailability of drugs and nutritional ... Several important drugs and nutritional supplements are limited by their lack of bioavailability.Nanomaterials display unique beneficial properties that might help improve the bioavailability of drugs and nutritional supplements.Unfortunately,nanomaterials produced from synthetic polymers and metals may have similar difficulties with bioavailability and toxicity.Naturally occurring biopolymers are biodegradable and non-toxic and are adaptable to the synthesis of nanoparticles.Drugs and other substances can be encapsulated or embedded in such particles with an increase in bioavailability.The search for biodegradable nanomaterials is an active research field.This review summarizes the research on nanocrystalline cellulose,starch,lignin,and other biological and environment-friendly nanocomposites which are commonly used as nanocarriers for drugs and nutrients.Further,prospects for the use of biodegradable nanomaterials in targeted therapy,including environmentally responsive therapy,are discussed. 展开更多
关键词 Nanomaterials biodegradation classification application
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Unraveling the interaction mechanism between enantiomers of lactone compounds(γ-octalactone andγ-undecalactone)in Longjing tea and OR1A1 olfactory receptor using molecular docking and molecular dynamics simulation 认领 引用 被引量：1
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作者 JianCai Zhu XiaoJie Liu +4 位作者 ZhenChun Sun TianYin Shen XingRan Kou YunWei Niu ZuoBing Xiao 《Food Bioscience》 SCIE 2025年第4期1659-1672,共14页
The interactions of key lactone chiral compounds(γ-octalactone andγ-undecalactone)in Longjing tea with olfactory receptors(taking OR1A1 as an example)were elucidated through molecular docking and molecular dynamics.... The interactions of key lactone chiral compounds(γ-octalactone andγ-undecalactone)in Longjing tea with olfactory receptors(taking OR1A1 as an example)were elucidated through molecular docking and molecular dynamics.The results showed that the thresholds forγ-octalactone,(R)-(+)-γ-octalactone,and(S)-(-)-γ-octalactone were 82μg/L,300μg/L,and 125μg/L,respectively.The thresholds forγ-undecalactone,(R)-(+)-γ-undecalactone and(S)-(-)-γ-undecalactone are 6μg/L,4μg/L,and 10μg/L,respectively.The binding of(S)-(-)-γ-octalactone(-18.389 kJ/mol)to the olfactory receptor OR1A1 is more stable than that of the(R)-(+)-γ-octalactone(-17.280 kJ/mol).On the contrary,(R)-(+)-γ-undecalactone(-19.146 kJ/mol)is binding stability than(S)-(-)-γ-undecalactone(-19.115 kJ/mol).Molecular dynamics simulations imply that the binding of(S)-(-)-γ-octalactone and(R)-(+)-γ-undecalactone to OR1A1 are primarily through polar and hydrogen bonding interactions,whereas(R)-(+)-γ-octalactone and(S)-(-)-γ-undecalactone are relies on hydrophobic interactions.These findings provide scientific support for improving the quality of Longjing tea. 展开更多
关键词 Lactone Chiral compounds Molecular docking Molecular dynamics simulation
The evaluation of interactions and molecular mechanisms between three acidic and sweet taste substances with sensory analysis,electronic tongue,and molecular dynamics simulation 认领 引用
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作者 Rujun Zhou Jiancai Zhu +5 位作者 Yuxin Li Yikai Hua Yunwei Niu Jing Zhang Zuobing Xiao Liming Zhao 《Food Bioscience》 SCIE 2025年第12期1932-1944,共13页
This study elucidates the modes of interaction and molecular mechanisms between three acidic substances(citric acid,malic acid,lactic acid)and sweet compounds(sucrose,glucose)through a multi-scale approach integrating... This study elucidates the modes of interaction and molecular mechanisms between three acidic substances(citric acid,malic acid,lactic acid)and sweet compounds(sucrose,glucose)through a multi-scale approach integrating sensory evaluation,electronic tongue analysis,and molecular simulations(docking and dynamics).The results revealed a concentration-dependent effect of acids on sweetness perception:at low concentrations(0.005-0.015%),a slight enhancement of sweetness was observed sensorially,while at higher concentrations(up to 0.025%),all three acids significantly could reduce perceived sweetness.The strength of suppression followed the order:citric acid>malic acid>lactic acid.Electronic tongue measurements demonstrated high consistency with sensory data,quantitatively confirming the antagonistic effect of acids on sweet taste perception by showing a significant decrease in sweetness response with increasing acid concentrations.Molecular docking and dynamics simulations indicated that acidic molecules competitively bind to the Venus flytrap domain(VFD)of the T1R2/T1R3 sweet receptor,disrupting sugar-receptor interactions.Citric acid,with three carboxyl groups,showed the strongest competitive binding,while lactic acid had the mildest effect due to its smaller size and reduced po-larity.This work provides a theoretical basis for the precise regulation of sweet-acid balance in beverage for-mulations,supporting the development of reduced-sugar products. 展开更多
关键词 Sour taste inhibition Sweet taste perception Sweet-acid interaction Molecular docking Electronic tongue
Molecular simulation analysis of differences in aroma synergy between three broad-spectrum proteins and four characteristic aroma compounds of sweet orange 认领 引用
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作者 ZhiMin Guo Qi Lu +5 位作者 YunWei Niu RuJun Zhou Jing Zhang JianCai Zhu ZuoBing Xiao Xiao Qing 《Food Bioscience》 SCIE 2025年第11期1626-1637,共12页
Sweet orange has become increasingly popular worldwide due to its unique flavor and nutritional value.In this study,four characteristic aroma compounds of sweet orange(α-pinene,octanal,ethyl butyrate,linalool)were se... Sweet orange has become increasingly popular worldwide due to its unique flavor and nutritional value.In this study,four characteristic aroma compounds of sweet orange(α-pinene,octanal,ethyl butyrate,linalool)were selected,and their interactions were evaluated at the macroscopic level through sensory experiments with pairwise combinations.Subsequently,the S-curve method combined with molecular simulation technology was used to systematically analyze the differences in synergistic effects between three broad-spectrum olfactory receptors(OR1A1,OR2W1,OR52D1)and the four characteristic aroma compounds of sweet orange.Sensory experiments showed that at least one masking effect existed in the pairwise combinations,and differences in aroma types led to different olfactory adaptation rates,with the synergistic effect betweenα-pinene and ethyl butyrate being particularly significant.Molecular docking revealed that hydrogen bonds in the active center of OR2W1(SER109/ASN155)and the multiple hydrogen bond network of OR1A1(THR239/SER/ARG122)were key binding modes,while OR52D1 had the weakest binding ability due to fewer and shorter hydrogen bonds.The rigid structure ofα-pinene caused steric hindrance,affecting the synergistic effect.Molecular dynamics further revealed that the high RMSD value of OR52D1 reflected its conformational flexibility,while OR2W1 enhanced binding stability through a“hydrophobic network”.This study confirms that olfactory perception is the result of hydrogen bonds,hydrophobic interactions,and dynamic equilibrium of molecular conformations,providing a theoretical basis for the synergistic mechanism of complex aroma systems. 展开更多
关键词 Characteristic aroma compounds of sweet orange Aroma synergy S-curve method Molecular simulation Interactions
Reactive mesoporous silica nanoparticles loaded with limonene for improving physical and mental health of mice at simulated microgravity condition 认领 引用 被引量：16
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作者 Zhiguo Lu Jianze Wang +9 位作者 Lina Qu Guanghan Kan Tianlu Zhang Jie Shen Yan Li Jun Yang Yunwei Niu Zuobing Xiao Yinghui Li Xin Zhang 《Bioactive Materials》 SCIE 2020年第4期1127-1137,共11页
Astronauts are under high stress for a long time because of the microgravity condition,which leads to anxiety,affects their learning and memory abilities,and seriously impairs the health of astronauts.Aromatherapy can... Astronauts are under high stress for a long time because of the microgravity condition,which leads to anxiety,affects their learning and memory abilities,and seriously impairs the health of astronauts.Aromatherapy can improve the physical and mental health of astronauts in a way that moisturizes them softly and silently.However,the strong volatility of fragrances and inconvenience of aroma treatment greatly limit their application in the field of spaceflight.In this study,reactive mesoporous silica nanoparticles were prepared to encapsulate and slowly release limonene.The limonene loaded nanoparticles were named limonene@mesoporous silica nanoparticles-cyanuric chloride(LE@MSNs-CYC).LE@MSNs-CYC were then applied to wallpaper to improve the convenience of aromatherapy.LE@MSNs-CYC could chemically react with the wallpaper,thus firmly adsorbed on the wallpaper.In the following,the mice were treated with hindlimb unloading(HU)to simulate a microgravity environment.The results showed that 28-day HU led to an increase in the level of anxiety and declines in learning,memory,and physical health in mice.LE@MSNs-CYC showed significant relief effects on anxiety,learning,memory,and physical health of HU treated mice.Subsequently,the molecular mechanisms were explored by hypothalamic-pituitary-adrenal axis related hormones,immune-related cytokines,learning,and memory-related neurotransmitters and proteins. 展开更多
关键词 Reactive mesoporous silica nanoparticles Slow release of limonene Simulated microgravity condition Improvement of physical health Improvement of mental health
Unraveling the characteristic aroma compounds in Longjing tea and their interaction mechanisms with S-curve and broad-spectrum olfactory receptors using molecular docking 认领 引用 被引量：15
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作者 ZuoBing Xiao TianYin Shen +6 位作者 YunWei Niu QinFei Ke ZhenChun Sun EnQing Yang XiaoJie Liu Jing Zhang JianCai Zhu 《Food Bioscience》 SCIE 2024年第4期1881-1895,共15页
The aroma of tea is one of the main sensory characteristics reflecting the quality of tea.The interactions between tea compounds were analyzed based on a S-curve method and molecular docking technology.This research e... The aroma of tea is one of the main sensory characteristics reflecting the quality of tea.The interactions between tea compounds were analyzed based on a S-curve method and molecular docking technology.This research examined the tea aroma intensity value before and after combination,the molecular docking energy through the predicted strength relationship,and the change of molecular docking energy and binding site to study compound interactions in the tea.The experiment showed that,according to the results of the determination of the sensory threshold value,the establishment of S-curve and the simulation calculation of molecular docking,the results of molecular docking and S-curve of the 10 characteristic compounds in tea selected in the present work reached the same conclusion.The results showed that studying the interaction of tea compounds based on molecular docking technology was simple,intuitive and reliable,which provided a theoretical basis and technical guidance for the study of the coordination action between compounds. 展开更多
关键词 S-curve method Molecular docking technology Tea Aroma compound
Green Fabrication of Multifunctional Three‑Dimensional Superabsorbent Nonwovens with Thermo‑Bonding Fibers 认领 引用 被引量：9
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作者 Jiajia Ma Nan Zhang +5 位作者 Ying Cheng Xingran Kou Yunwei Niu Xiangyu Jin Qinfei Ke Yi Zhao 《Advanced Fiber Materials》 SCIE EI CAS 2022年第2期293-304,共12页
Disposable hygiene products have evolved into the important parts for millions of people around the world,enhancing the convenience of daily lives.However,development of the disposable hygiene products is restricted b... Disposable hygiene products have evolved into the important parts for millions of people around the world,enhancing the convenience of daily lives.However,development of the disposable hygiene products is restricted by unsustainable production technology,complicated operation process,and poor liquid absorption performance of the absorbent core.Herein,integrated and three-dimensional(3D)multifunctional superabsorbent nonwovens with liquid-triggered fragrance release was prepared via green,fast and scalable multi efect hot-air anchoring method which physically crosslinking the joint thermobonding fbers and anchoring fragrance microcapsules/super absorbent polymer(SAP)onto adjacent thermo-bonding fbers simultaneously.The resulting composite nonwovens could three-dimensionally absorb water 33.14 times of its own weight without gel blockage between SAP,and correspondingly release increased intensity fragrance along with enhancing amount of water absorption.Absorption rate t1 and t2 is 83.62%and 50.62%higher than the commercial specimen respectively,and the air permeability is increased by 226.88%compared with the commercial specimen.The superabsorbent nonwovens with controllable fragrance release and odorant synergistic has the potential to be practically applied to functional textiles felds because of the excellent liquid absorption and controlled fragrance release performance,and is easy to be produced on a sustainable,pollution-free and large-scale industrial production. 展开更多
关键词 3D superabsorbent nonwovens Hot-air anchoring Thermo-bonding fber Without gel blockage Controlled fragrance release Environmentally friendly
Formation of fluorescent substances and correlation with process flavor changes of dehydrated Maillard reaction intermediates of peanut protein hydrolysates 认领 引用 被引量：2
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作者 Wenyu Zhou Cheng Huang +7 位作者 Yishun Yao Tong Zhou Heping Cui Yunwei Niu Foxin Zhang Khizar Hayat Xiaoming Zhang Chi-Tang Ho 《Food Bioscience》 SCIE 2023年第6期2599-2608,共10页
Maillard reaction intermediates(MRIs)derived from peanut protein hydrolysates(PPH)and xylose(Xyl)were prepared using the water bath combined with spray drying and vacuum drying.The monitoring of free amino content,bro... Maillard reaction intermediates(MRIs)derived from peanut protein hydrolysates(PPH)and xylose(Xyl)were prepared using the water bath combined with spray drying and vacuum drying.The monitoring of free amino content,browning precursors,and taste characteristics was carried out throughout the thermal treatment at low temperature,where the Maillard reaction process was slowed down,and the formation and degradation of MRIs were dynamically balanced at low conversion rates.The reaction between amino compounds and the reducing sugars contributed to the increased taste characteristics during the early phase of Maillard reaction.Fluorescence intensity was reduced after reaching its maximum value and browning intensity was significantly increased during vacuum drying,which confirmed that the Maillard reaction entered into an advanced stage.Vacuum drying also led to a significant increase in the total amount of volatile compounds in the subsequent thermal processing reaction(from 212.93 ng/g to 564.91 ng/g),which demonstrated that the higher fluorescence intensities resulted in the more accumulation of MRIs and better capabilities of flavor formation. 展开更多
关键词 Peanut protein Fluorescence spectroscopy Free amino group Saltiness enhancement Volatile compounds
Preparation of umami peptides from chicken breast by ultrasound-assisted gradient dilution feeding substrate and study of their formation mechanism 认领 引用 被引量：1
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作者 Jing Guo Xiaojie Yu +8 位作者 Cunshan Zhou Bo Wang Lei Zhang Phyllis Otu Li Chen Yunwei Niu Deyang Yao Chenhui Hua Haile Ma 《Food Bioscience》 SCIE 2024年第6期2759-2767,共9页
Gradient dilution feeding substrate(GDFS)is regarded as an effective method for the production of active peptides,as it compensates for substrate limitations and minimizes substrate contamination of the ultrafiltratio... Gradient dilution feeding substrate(GDFS)is regarded as an effective method for the production of active peptides,as it compensates for substrate limitations and minimizes substrate contamination of the ultrafiltration membrane.This study further investigated the impact of ultrasound-assisted gradient dilution feeding substrate(UA-GDFS)on the peptide yield and the intensity of umami.The chicken breast was used as ingredients.The umami compounds in the hydrolysate were determined using an automatic amino acid analyzer and HPLC.The hydrolysate’s umami intensity was determined by electronic tongue in all modes.These findings indicated that UA-GDFS enhanced the umami intensity and peptide yield.Hydrolysate from UA-GDFS with molecular weight below 1 kDa was analyzed by nano-scale liquid chromatography-tandem mass spectrometry(Nano-HPLC-MS/MS).Electronic tongue analysis showed that GPSGPVG and VDGPSGK had umami taste and could enhance the umami taste of monosodium glutamate(MSG)solution.Asn68 and His145 were important sites on T1R3 for umami peptide binding. 展开更多
关键词 Chicken breast Ultrasound-assisted Feeding substrate Nano-HPLC-MS/MS Umami peptides Molecular docking
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